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Paulo Tomé
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We maybe need to use "unified cgroup hierarchy" as explained at Unified and Legacy Control Group Hierarchies.

To enable this feature, add systemd.unified_cgroup_hierarchy=1 to GRUB_CMDLINE_LINUX_DEFAULT in /etc/default/grub, run update-grub, and reboot Linux.

systemd.unified_cgroup_hierarchy is explained insystemd unified cgroup hierarchy.

Then added the following lines at [Service] section of your systemd unit file, and run systemctl daemon-reload:

Delegate=memory
MemoryHigh=8G (if you choose 8 gigabytes as the limit)

Explanation of "MemoryHigh" is given at systemd.resource-control.